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Theory of non-linear susceptibility and correlation length in glasses and liquids

  • Claudio Donati
  • , Silvio Franz*
  • , Sharon C. Glotzer
  • , Giorgio Parisi
  • *此作品的通讯作者

科研成果: 期刊稿件文章同行评审

摘要

Within the framework of the effective potential theory of the structural glass transition, we calculate for the p-spin model and for a hard sphere liquid in the hypernetted chain approximation a static non-linear susceptibility related to a four-point density correlation function, and show that it diverges in mean field with exponent γ = 1/2 as the critical temperature Tc is approached from below. When Tc is approached from above, we calculate for the p-spin model a time dependent non-linear susceptibility and show that there is a characteristic time where this susceptibility has a maximum, and that this time grows with decreasing T. This susceptibility diverges as Tc is approached from above, and has key features in common with a generalized susceptibility related to particle displacements, previously introduced to measure correlated particle motion in simulations of glass-forming liquids.

源语言英语
页(从-至)215-224
页数10
期刊Journal of Non-Crystalline Solids
307-310
DOI
出版状态已出版 - 9月 2002
已对外发布

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