Mechanically Robust and Broadband Blackbody Composite Films Based on Self-Assembled Layered Structures

Inspired by nacre that is mechanically strong and versatile in light manipulation, large-scale black films with a nacre-like microstructure and carbon nanotube inclusion were prepared using a facile self-assembly technique. A layered structure promoting blackness and toughness simultaneously was realized, affording robust films with a solar–absorptivity as high as 96.9%. Our design strategy and fabrication process will be beneficial for the facile access to various advanced blackbody coatings.