TY - JOUR
T1 - High-Performance NH3 Sensors Based on Surface Modification by Plasma and Irradiation at Room Temperature
AU - Liu, Han
AU - Han, Han
AU - Li, He Guo
AU - Zhang, Shou Xin
AU - Li, Xiao Peng
AU - Yue, Yi Yu
AU - Wang, Ming Qing
AU - Zhao, Yue
AU - Fan, Zhi Qiang
N1 - Publisher Copyright:
© 2025 The Authors. Published by American Chemical Society.
PY - 2025/6/24
Y1 - 2025/6/24
N2 - In this paper, we investigated the sensor characteristics of gas-sensitive sensors with the structure of rGO sprayed onto interdigital electrodes under test conditions of room temperature and 47.2% RH (relative humidity), which were obtained through the surface modification methods of plasma treatment and irradiation treatment. First, we prepared a batch of sensors through experimental procedures and then obtained sensors with good gas-sensitive performance by varying the heating temperature of the sensors and the channel width of the interdigital electrodes. Second, plasma surface modification was utilized to enhance the sensitivity of the sensors. Third, irradiation modification was implemented to improve the sensor performance, including response and recovery times as well as sensitivity. Moreover, the response and recovery curves of the sensors under different NH3 gas concentrations were measured. It was found that the two surface modification methods, plasma treatment and surface irradiation treatment, have a prominent impact on the improvement of response and recovery times and sensitivity in the sensor. In addition, we tested the selectivity and repeatability of the sensor and found that the sensor was more selective for NH3 compared to NO2, and has excellent repeatability. Finally, we fully characterized the material to explore the mechanism.
AB - In this paper, we investigated the sensor characteristics of gas-sensitive sensors with the structure of rGO sprayed onto interdigital electrodes under test conditions of room temperature and 47.2% RH (relative humidity), which were obtained through the surface modification methods of plasma treatment and irradiation treatment. First, we prepared a batch of sensors through experimental procedures and then obtained sensors with good gas-sensitive performance by varying the heating temperature of the sensors and the channel width of the interdigital electrodes. Second, plasma surface modification was utilized to enhance the sensitivity of the sensors. Third, irradiation modification was implemented to improve the sensor performance, including response and recovery times as well as sensitivity. Moreover, the response and recovery curves of the sensors under different NH3 gas concentrations were measured. It was found that the two surface modification methods, plasma treatment and surface irradiation treatment, have a prominent impact on the improvement of response and recovery times and sensitivity in the sensor. In addition, we tested the selectivity and repeatability of the sensor and found that the sensor was more selective for NH3 compared to NO2, and has excellent repeatability. Finally, we fully characterized the material to explore the mechanism.
UR - https://www.scopus.com/pages/publications/105007907167
U2 - 10.1021/acsomega.5c01879
DO - 10.1021/acsomega.5c01879
M3 - 文章
AN - SCOPUS:105007907167
SN - 2470-1343
VL - 10
SP - 25775
EP - 25789
JO - ACS Omega
JF - ACS Omega
IS - 24
ER -