TY - JOUR
T1 - Hierarchically-structured light-thermal solid slippery interface for anti-/de-icing
AU - Zhao, Di
AU - Sun, Xu
AU - Chai, Ziyuan
AU - Chi, Chengcheng
AU - Zuo, Xiaobiao
AU - Jiang, Lei
AU - Heng, Liping
N1 - Publisher Copyright:
© 2025 Elsevier B.V.
PY - 2025/6/1
Y1 - 2025/6/1
N2 - Ice formation in harsh weather conditions poses a significant challenge across various sectors, including transportation, energy, and infrastructure. Researchers have recently developed a variety of solar-driven photothermal slippery interfaces for deicing applications, showcasing excellent anti-icing and de-icing capabilities. However, these interfaces often suffer from low solar efficiency and require high operating temperatures, primarily due to suboptimal photothermal layer design, hindering their broad application. To address these issues, we developed a hierarchically structured photothermal solid slippery interface (P/HPC), consisting of paraffin, polydimethylsiloxane (PDMS), and carbon black, using a double-template method. The unique micro/nano hierarchical porous structure of the photothermal layer promotes multiple internal reflections of sunlight, thereby enhancing solar absorption and exhibiting superior photothermal properties. Under 1.0 kW/m2 light intensity, this composite interface demonstrates exceptional anti-/de-icing properties, even at temperatures as low as −50 °C. Moreover, the interface demonstrates outstanding light-triggered self-healing abilities and stability under harsh conditions, offering a promising solution for anti-/de-icing applications in a variety of extreme environments.
AB - Ice formation in harsh weather conditions poses a significant challenge across various sectors, including transportation, energy, and infrastructure. Researchers have recently developed a variety of solar-driven photothermal slippery interfaces for deicing applications, showcasing excellent anti-icing and de-icing capabilities. However, these interfaces often suffer from low solar efficiency and require high operating temperatures, primarily due to suboptimal photothermal layer design, hindering their broad application. To address these issues, we developed a hierarchically structured photothermal solid slippery interface (P/HPC), consisting of paraffin, polydimethylsiloxane (PDMS), and carbon black, using a double-template method. The unique micro/nano hierarchical porous structure of the photothermal layer promotes multiple internal reflections of sunlight, thereby enhancing solar absorption and exhibiting superior photothermal properties. Under 1.0 kW/m2 light intensity, this composite interface demonstrates exceptional anti-/de-icing properties, even at temperatures as low as −50 °C. Moreover, the interface demonstrates outstanding light-triggered self-healing abilities and stability under harsh conditions, offering a promising solution for anti-/de-icing applications in a variety of extreme environments.
KW - Anti-/de-icing
KW - Hierarchical porous structures
KW - Photothermal slippery interfaces
KW - Self-healing
KW - Solid slippery interfaces
UR - https://www.scopus.com/pages/publications/105003147182
U2 - 10.1016/j.cej.2025.162943
DO - 10.1016/j.cej.2025.162943
M3 - 文章
AN - SCOPUS:105003147182
SN - 1385-8947
VL - 513
JO - Chemical Engineering Journal
JF - Chemical Engineering Journal
M1 - 162943
ER -