Abstract
Solution-processed lead halide perovskites are considered one of the promising materials for flexible optoelectronics. However, the array integration of ultrathin flexible perovskite photodetectors (PDs) remains a significant challenge limited by the incompatibility of perovskite materials with manufacturing techniques involving polar liquids. Here, an ultrathin (2.4 µm) and conformable perovskite-based PD array (10 × 10 pixels) with ultralight weight (3.12 g m−2) and excellent flexibility, is reported. Patterned all-inorganic CsPbBr3 perovskite films with precise pixel position, controllable morphology, and homogenous dimension, are synthesized by a vacuum-assisted drop-casting patterning process as the active layer. The use of waterproof parylene-C film as substrate and encapsulation layer effectively protects the perovskite films against penetration of polar liquids during the peeling-off process. Benefitting from the encapsulation and ultrathin property, the device exhibits long-term stability in the ambient environment, and robust mechanical stability under bending or 50% compressive strain. More importantly, the ultrathin flexible PD arrays conforming to hemispherical support realize imaging of light distribution, indicating the potential applications in retina-like vision sensing.
| Original language | English |
|---|---|
| Article number | 2006006 |
| Journal | Advanced Materials |
| Volume | 33 |
| Issue number | 9 |
| DOIs | |
| State | Published - 4 Mar 2021 |
| Externally published | Yes |
Keywords
- all-inorganic CsPbBr perovskite
- artificial vision sensing
- conformable contact
- photodetector arrays
- ultrathin photodetectors
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