Abstract
Due to thermionic emission of triboelectric charge and degradation of mechanical stability of polymer tribomaterials (PTMs), PTMs based TENG (PTM-TENG) cannot maintain efficient electrical output and operate stably at high temperatures. Herein, a series of fatty acid doped PVDF-HFP (PH-FA) PTMs are fabricated. The introduction of FA lubricants dramatically increases the β-phase relative fraction, dielectric constant and surface charge potential of PTMs. Therefore, the PH-SA (stearic acid) based TENG shows improved electrical output over a wide temperature range, extraordinary stability, and durability. Particularly, the VT/VRoom, IT/IRoom and QT/QRoom of PH-SA at 100 °C are separately up to 231.10%, 251.46% and 234.01%, the output efficiency of PH-SA is still higher than 100% at 120 °C. This study not only provides pioneering reference for the development of advanced PTM-TENG with enhanced output performance over a wide temperature range, but also greatly promotes the application of PTM-TENG devices in harsh environments.
| Original language | English |
|---|---|
| Article number | 108347 |
| Journal | Nano Energy |
| Volume | 110 |
| DOIs | |
| State | Published - 1 Jun 2023 |
| Externally published | Yes |
UN SDGs
This output contributes to the following UN Sustainable Development Goals (SDGs)
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SDG 7 Affordable and Clean Energy
Keywords
- Enhanced electrical output
- Fatty acid
- High temperature
- Polymer tribomaterials
- Stability
- Triboelectric nanogenerator
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