Suppressing strain propagation in ultrahigh-Ni cathodes during fast charging via epitaxial entropy-assisted coating

Chen Zhao; Chuanwei Wang; Xiang Liu; Inhui Hwang; Tianyi Li; Xinwei Zhou; Jiecheng Diao; Junjing Deng; Yan Qin; Zhenzhen Yang; Guanyi Wang; Wenqian Xu; Chengjun Sun; Longlong Wu; Wonsuk Cha; Ian Robinson; Ross Harder; Yi Jiang; Tekin Bicer; Jun Tao Li; Wenquan Lu; Luxi Li; Yuzi Liu; Shi Gang Sun; Gui Liang Xu; Khalil Amine

doi:10.1038/s41560-024-01465-2

Suppressing strain propagation in ultrahigh-Ni cathodes during fast charging via epitaxial entropy-assisted coating

Chen Zhao
, Chuanwei Wang
, Xiang Liu
, Inhui Hwang
, Tianyi Li
, Xinwei Zhou
, Jiecheng Diao
, Junjing Deng
, Yan Qin
, Zhenzhen Yang
, Guanyi Wang
, Wenqian Xu
, Chengjun Sun
, Longlong Wu
, Wonsuk Cha
, Ian Robinson
, Ross Harder
, Yi Jiang
, Tekin Bicer
, Jun Tao Li

Wenquan Lu, Luxi Li^*, Yuzi Liu^*, Shi Gang Sun, Gui Liang Xu^*, Khalil Amine^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

155 Scopus citations

Abstract

Layered Ni-rich oxide cathodes are susceptible to challenges with surface reconstruction and strain propagation, limiting their cyclability. The authors propose a solution involving oriented attachment-driven reactions, utilizing Wadsley–Roth nanocrystals and layered oxide to induce an epitaxial entropy-assisted coating, effectively addressing these issues.

Original language	English
Pages (from-to)	345-356
Number of pages	12
Journal	Nature Energy
Volume	9
Issue number	3
DOIs	https://doi.org/10.1038/s41560-024-01465-2
State	Published - Mar 2024
Externally published	Yes

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SDG 7 Affordable and Clean Energy

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10.1038/s41560-024-01465-2

Cite this

Zhao, C., Wang, C., Liu, X., Hwang, I., Li, T., Zhou, X., Diao, J., Deng, J., Qin, Y., Yang, Z., Wang, G., Xu, W., Sun, C., Wu, L., Cha, W., Robinson, I., Harder, R., Jiang, Y., Bicer, T., ... Amine, K. (2024). Suppressing strain propagation in ultrahigh-Ni cathodes during fast charging via epitaxial entropy-assisted coating. Nature Energy, 9(3), 345-356. https://doi.org/10.1038/s41560-024-01465-2

@article{0ae13ef61d664185a49f39c73b623904,

title = "Suppressing strain propagation in ultrahigh-Ni cathodes during fast charging via epitaxial entropy-assisted coating",

abstract = "Layered Ni-rich oxide cathodes are susceptible to challenges with surface reconstruction and strain propagation, limiting their cyclability. The authors propose a solution involving oriented attachment-driven reactions, utilizing Wadsley–Roth nanocrystals and layered oxide to induce an epitaxial entropy-assisted coating, effectively addressing these issues.",

author = "Chen Zhao and Chuanwei Wang and Xiang Liu and Inhui Hwang and Tianyi Li and Xinwei Zhou and Jiecheng Diao and Junjing Deng and Yan Qin and Zhenzhen Yang and Guanyi Wang and Wenqian Xu and Chengjun Sun and Longlong Wu and Wonsuk Cha and Ian Robinson and Ross Harder and Yi Jiang and Tekin Bicer and Li, \{Jun Tao\} and Wenquan Lu and Luxi Li and Yuzi Liu and Sun, \{Shi Gang\} and Xu, \{Gui Liang\} and Khalil Amine",

note = "Publisher Copyright: {\textcopyright} The Author(s), under exclusive licence to Springer Nature Limited 2024. corrected publication 2024..",

year = "2024",

month = mar,

doi = "10.1038/s41560-024-01465-2",

language = "英语",

volume = "9",

pages = "345--356",

journal = "Nature Energy",

issn = "2058-7546",

publisher = "Springer Nature",

number = "3",

}

Zhao, C, Wang, C, Liu, X, Hwang, I, Li, T, Zhou, X, Diao, J, Deng, J, Qin, Y, Yang, Z, Wang, G, Xu, W, Sun, C, Wu, L, Cha, W, Robinson, I, Harder, R, Jiang, Y, Bicer, T, Li, JT, Lu, W, Li, L, Liu, Y, Sun, SG, Xu, GL & Amine, K 2024, 'Suppressing strain propagation in ultrahigh-Ni cathodes during fast charging via epitaxial entropy-assisted coating', Nature Energy, vol. 9, no. 3, pp. 345-356. https://doi.org/10.1038/s41560-024-01465-2

TY - JOUR

T1 - Suppressing strain propagation in ultrahigh-Ni cathodes during fast charging via epitaxial entropy-assisted coating

AU - Zhao, Chen

AU - Wang, Chuanwei

AU - Liu, Xiang

AU - Hwang, Inhui

AU - Li, Tianyi

AU - Zhou, Xinwei

AU - Diao, Jiecheng

AU - Deng, Junjing

AU - Qin, Yan

AU - Yang, Zhenzhen

AU - Wang, Guanyi

AU - Xu, Wenqian

AU - Sun, Chengjun

AU - Wu, Longlong

AU - Cha, Wonsuk

AU - Robinson, Ian

AU - Harder, Ross

AU - Jiang, Yi

AU - Bicer, Tekin

AU - Li, Jun Tao

AU - Lu, Wenquan

AU - Li, Luxi

AU - Liu, Yuzi

AU - Sun, Shi Gang

AU - Xu, Gui Liang

AU - Amine, Khalil

N1 - Publisher Copyright: © The Author(s), under exclusive licence to Springer Nature Limited 2024. corrected publication 2024..

PY - 2024/3

Y1 - 2024/3

N2 - Layered Ni-rich oxide cathodes are susceptible to challenges with surface reconstruction and strain propagation, limiting their cyclability. The authors propose a solution involving oriented attachment-driven reactions, utilizing Wadsley–Roth nanocrystals and layered oxide to induce an epitaxial entropy-assisted coating, effectively addressing these issues.

AB - Layered Ni-rich oxide cathodes are susceptible to challenges with surface reconstruction and strain propagation, limiting their cyclability. The authors propose a solution involving oriented attachment-driven reactions, utilizing Wadsley–Roth nanocrystals and layered oxide to induce an epitaxial entropy-assisted coating, effectively addressing these issues.

UR - https://www.scopus.com/pages/publications/85186224978

U2 - 10.1038/s41560-024-01465-2

DO - 10.1038/s41560-024-01465-2

M3 - 文章

AN - SCOPUS:85186224978

SN - 2058-7546

VL - 9

SP - 345

EP - 356

JO - Nature Energy

JF - Nature Energy

IS - 3

ER -

Suppressing strain propagation in ultrahigh-Ni cathodes during fast charging via epitaxial entropy-assisted coating

Abstract

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