Hydrotreatment of Jatropha oil over NiMoLa/Al2O3 catalyst

Jing Liu; Can Liu; Gang Zhou; Shituan Shen; Long Rong

doi:10.1039/c2gc35450k

Hydrotreatment of Jatropha oil over NiMoLa/Al₂O₃ catalyst

Jing Liu
, Can Liu
, Gang Zhou
, Shituan Shen
, Long Rong^*

^*Corresponding author for this work

School of Biological Science and Medical Engineering

Beihang University

Research output: Contribution to journal › Article › peer-review

88 Scopus citations

Abstract

The non-sulfided NiMoLa/Al₂O₃ catalyst was developed to produce renewable C₁₅-C₁₈ alkanes from the hydrotreatment of Jatropha oil. The NiMoLa/Al₂O₃ catalysts were prepared by an impregnation method and characterized by N₂-BET, XRD, XPS, TPD-H_ads, CO₂-TPD and TGA techniques. The straight chain alkanes ranging from C₁₅ to C₁₈ were the main components in the product oil. A yield of 78%, a selectivity of 94% and a conversion of 83% were obtained at 370 °C, 3.5 MPa and 0.9 h^-1 over the NiMoLa/Al₂O₃ catalyst (La 5.0 wt%). The influence of the reaction temperature (280-400 °C) and reaction time (4-177 h) on the composition of product oil were also investigated.

Original language	English
Pages (from-to)	2499-2505
Number of pages	7
Journal	Green Chemistry
Volume	14
Issue number	9
DOIs	https://doi.org/10.1039/c2gc35450k
State	Published - Sep 2012

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title = "Hydrotreatment of Jatropha oil over NiMoLa/Al2O3 catalyst",

abstract = "The non-sulfided NiMoLa/Al2O3 catalyst was developed to produce renewable C15-C18 alkanes from the hydrotreatment of Jatropha oil. The NiMoLa/Al2O3 catalysts were prepared by an impregnation method and characterized by N2-BET, XRD, XPS, TPD-Hads, CO2-TPD and TGA techniques. The straight chain alkanes ranging from C15 to C18 were the main components in the product oil. A yield of 78\%, a selectivity of 94\% and a conversion of 83\% were obtained at 370 °C, 3.5 MPa and 0.9 h-1 over the NiMoLa/Al2O3 catalyst (La 5.0 wt\%). The influence of the reaction temperature (280-400 °C) and reaction time (4-177 h) on the composition of product oil were also investigated.",

author = "Jing Liu and Can Liu and Gang Zhou and Shituan Shen and Long Rong",

year = "2012",

month = sep,

doi = "10.1039/c2gc35450k",

language = "英语",

volume = "14",

pages = "2499--2505",

journal = "Green Chemistry",

issn = "1463-9262",

publisher = "Royal Society of Chemistry",

number = "9",

}

TY - JOUR

T1 - Hydrotreatment of Jatropha oil over NiMoLa/Al2O3 catalyst

AU - Liu, Jing

AU - Liu, Can

AU - Zhou, Gang

AU - Shen, Shituan

AU - Rong, Long

PY - 2012/9

Y1 - 2012/9

N2 - The non-sulfided NiMoLa/Al2O3 catalyst was developed to produce renewable C15-C18 alkanes from the hydrotreatment of Jatropha oil. The NiMoLa/Al2O3 catalysts were prepared by an impregnation method and characterized by N2-BET, XRD, XPS, TPD-Hads, CO2-TPD and TGA techniques. The straight chain alkanes ranging from C15 to C18 were the main components in the product oil. A yield of 78%, a selectivity of 94% and a conversion of 83% were obtained at 370 °C, 3.5 MPa and 0.9 h-1 over the NiMoLa/Al2O3 catalyst (La 5.0 wt%). The influence of the reaction temperature (280-400 °C) and reaction time (4-177 h) on the composition of product oil were also investigated.

AB - The non-sulfided NiMoLa/Al2O3 catalyst was developed to produce renewable C15-C18 alkanes from the hydrotreatment of Jatropha oil. The NiMoLa/Al2O3 catalysts were prepared by an impregnation method and characterized by N2-BET, XRD, XPS, TPD-Hads, CO2-TPD and TGA techniques. The straight chain alkanes ranging from C15 to C18 were the main components in the product oil. A yield of 78%, a selectivity of 94% and a conversion of 83% were obtained at 370 °C, 3.5 MPa and 0.9 h-1 over the NiMoLa/Al2O3 catalyst (La 5.0 wt%). The influence of the reaction temperature (280-400 °C) and reaction time (4-177 h) on the composition of product oil were also investigated.

UR - https://www.scopus.com/pages/publications/84868198298

U2 - 10.1039/c2gc35450k

DO - 10.1039/c2gc35450k

M3 - 文章

AN - SCOPUS:84868198298

SN - 1463-9262

VL - 14

SP - 2499

EP - 2505

JO - Green Chemistry

JF - Green Chemistry

IS - 9

ER -

Hydrotreatment of Jatropha oil over NiMoLa/Al₂O₃ catalyst

Abstract

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