Highly efficient non-precious metal electrocatalysts prepared from one-pot synthesized zeolitic imidazolate frameworks

Dan Zhao; Jiang Lan Shui; Lauren R. Grabstanowicz; Chen Chen; Sean M. Commet; Tao Xu; Jun Lu; Di Jia Liu

doi:10.1002/adma.201304238

Highly efficient non-precious metal electrocatalysts prepared from one-pot synthesized zeolitic imidazolate frameworks

Dan Zhao
, Jiang Lan Shui
, Lauren R. Grabstanowicz
, Chen Chen
, Sean M. Commet
, Tao Xu
, Jun Lu
, Di Jia Liu^*

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

302 Scopus citations

Abstract

A facile synthesis of non-PGM ORR electrocatalysts through thermolysis of one-pot synthesized ZIF is demonstrated. The electrocatalysts exhibit excellent activity, with a maximum volumetric current density of 88.1 A cm^-3 measured at 0.8 V in PEFC tests. This approach not only makes ZIFs-based electrocatalysts easy to scale up, but also paves the way for the tailored synthesis of electrocatalysts.

Original language	English
Pages (from-to)	1093-1097
Number of pages	5
Journal	Advanced Materials
Volume	26
Issue number	7
DOIs	https://doi.org/10.1002/adma.201304238
State	Published - 19 Feb 2014
Externally published	Yes

Keywords

catalysis
fuel cells
metal-organic frameworks
oxygen reduction reactions
solid-state synthesis

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10.1002/adma.201304238

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title = "Highly efficient non-precious metal electrocatalysts prepared from one-pot synthesized zeolitic imidazolate frameworks",

abstract = "A facile synthesis of non-PGM ORR electrocatalysts through thermolysis of one-pot synthesized ZIF is demonstrated. The electrocatalysts exhibit excellent activity, with a maximum volumetric current density of 88.1 A cm-3 measured at 0.8 V in PEFC tests. This approach not only makes ZIFs-based electrocatalysts easy to scale up, but also paves the way for the tailored synthesis of electrocatalysts.",

keywords = "catalysis, fuel cells, metal-organic frameworks, oxygen reduction reactions, solid-state synthesis",

author = "Dan Zhao and Shui, \{Jiang Lan\} and Grabstanowicz, \{Lauren R.\} and Chen Chen and Commet, \{Sean M.\} and Tao Xu and Jun Lu and Liu, \{Di Jia\}",

year = "2014",

month = feb,

day = "19",

doi = "10.1002/adma.201304238",

language = "英语",

volume = "26",

pages = "1093--1097",

journal = "Advanced Materials",

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T1 - Highly efficient non-precious metal electrocatalysts prepared from one-pot synthesized zeolitic imidazolate frameworks

AU - Zhao, Dan

AU - Shui, Jiang Lan

AU - Grabstanowicz, Lauren R.

AU - Chen, Chen

AU - Commet, Sean M.

AU - Xu, Tao

AU - Lu, Jun

AU - Liu, Di Jia

PY - 2014/2/19

Y1 - 2014/2/19

N2 - A facile synthesis of non-PGM ORR electrocatalysts through thermolysis of one-pot synthesized ZIF is demonstrated. The electrocatalysts exhibit excellent activity, with a maximum volumetric current density of 88.1 A cm-3 measured at 0.8 V in PEFC tests. This approach not only makes ZIFs-based electrocatalysts easy to scale up, but also paves the way for the tailored synthesis of electrocatalysts.

AB - A facile synthesis of non-PGM ORR electrocatalysts through thermolysis of one-pot synthesized ZIF is demonstrated. The electrocatalysts exhibit excellent activity, with a maximum volumetric current density of 88.1 A cm-3 measured at 0.8 V in PEFC tests. This approach not only makes ZIFs-based electrocatalysts easy to scale up, but also paves the way for the tailored synthesis of electrocatalysts.

KW - catalysis

KW - fuel cells

KW - metal-organic frameworks

KW - oxygen reduction reactions

KW - solid-state synthesis

UR - https://www.scopus.com/pages/publications/84894288988

U2 - 10.1002/adma.201304238

DO - 10.1002/adma.201304238

M3 - 文章

AN - SCOPUS:84894288988

SN - 0935-9648

VL - 26

SP - 1093

EP - 1097

JO - Advanced Materials

JF - Advanced Materials

IS - 7

ER -

Highly efficient non-precious metal electrocatalysts prepared from one-pot synthesized zeolitic imidazolate frameworks

Abstract

Keywords

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