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Heavy metal removal from aqueous solutions by calcium silicate powder from waste coal fly-ash

  • Jing Ma
  • , Guotong Qin*
  • , Yupei Zhang
  • , Junmin Sun
  • , Shuli Wang
  • , Lei Jiang
  • *Corresponding author for this work
  • Beihang University
  • National Energy Key Laboratory on Development and Utilization of High Alumina Coal Resources

Research output: Contribution to journalArticlepeer-review

Abstract

The removal of Ni (II), Cu (II), Zn (II), and Co (II) ions from simulated aqueous solutions using calcium silicate powder (CSP), a new by-product derived from the production of alumina from coal ash, has been studied. CSP showed high efficiency for the removal of these metal ions. The maximum adsorptions were 420.17, 680.93, 251.89, and 235.29 mg/g for Ni (II), Cu (II), Zn (II), and Co (II), respectively. Total (100%) removal of Ni (II) was obtained when the initial concentration was 100 mg/L, indicating that CSP was highly effective even at an extremely low concentration. Adsorption isotherms and kinetics have been studied using different models. It has been found that the adsorption isotherms can best be described on the basis of the Langmuir model, with the kinetics of adsorption following a pseudo-second-order reaction process. The calcium ion concentration was examined before and after adsorption to investigate the mechanism of removal of the heavy metal ions. It was found that the removal of heavy metal ions is mainly achieved through ion-exchange, combined with some adsorption.

Original languageEnglish
Pages (from-to)776-782
Number of pages7
JournalJournal of Cleaner Production
Volume182
DOIs
StatePublished - 1 May 2018

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

  1. SDG 7 - Affordable and Clean Energy
    SDG 7 Affordable and Clean Energy

Keywords

  • Adsorption
  • Calcium silicate powder
  • Heavy metal
  • Mechanism

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