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A DFT study on graphene-based surface-enhanced Raman spectroscopy of Benzenedithiol adsorbed on gold/graphene

  • Beihang University

Research output: Contribution to journalArticlepeer-review

Abstract

In this study, a detailed analysis on the surface-enhanced Raman scattering of 1,4-Benzenedithiol adsorbed on gold/graphene cluster is presented by density functional theory calculations. Results indicate that changing graphene type including perfect graphene, monovacancy graphene, B/N-doped grapheme, and graphene oxide enables modulation of interaction between molecule, gold, and graphene cluster. Calculated Raman spectra of surface complexes are discussed considering chemical enhancement for graphene-based surface-enhanced Raman scattering study, which shows dependence on graphene types, which is related to several influence factors from electronic structure to excitation properties.

Original languageEnglish
Pages (from-to)1510-1518
Number of pages9
JournalJournal of Raman Spectroscopy
Volume50
Issue number10
DOIs
StatePublished - 1 Oct 2019

Keywords

  • 1,4-Benzenedithiol
  • DFT
  • SERS
  • gold
  • graphene

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